WordPress themes and Vanilla themes are completely independent.
You can, of course, copy the look of an existing theme from any site. You basically just take the CSS from that site and map the selectors to their semantic equivalents of Vanilla. @whu606 wrote an annotated theme that would help you in this case: http://vanillaforums.org/addon/annotatedcss2.1-theme
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WordPress themes and Vanilla themes are completely independent.
You can, of course, copy the look of an existing theme from any site. You basically just take the CSS from that site and map the selectors to their semantic equivalents of Vanilla. @whu606 wrote an annotated theme that would help you in this case: http://vanillaforums.org/addon/annotatedcss2.1-theme
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there is a plugin for integration